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Are they textbooks, or just books that were used in psych classes? (Generally, libraries aren't interested in textbooks)
You're probably not going to find any interest in old textbooks (especially if they've been superseded by later editions. But yeah, you could donate to a public library, they'll slide them down to the "Friends of..." organization which will try to sell them at the annual sale and then they'll be offered to prisons and jails and if after that nobody wants them they'll go in the trash (though people find it scandalous for some reason, libraries put a lot of books in the trash ultimately).
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