One thing to keep in mind is what is being done with the artwork after it is created. If this is going to be printed (in a book/magazine/brochure/etc.) you want to stay away from raster based graphics (which I believe Paint works strictly in - though I may be wrong).
Also, if this is going to print (again - I am not talking about your ink-jet printer; I am talking about offset litho printing), try to work in a CMYK color space, not RGB. You want to make sure that what you are creating can be reproduced!
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